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Predicting the formation of mud cracks in Li-ion battery electrodes during the drying process with in situ X-ray computed tomography

Will J. Dawson, Andrew R. T. Morrison, Simon M. Tonge, Matthew P. Jones, Kofi Coke, Isabel C. Antony, Kaz Wanelik, Vyacheslav Kachkanov, Partha P. Paul, Bratislav Lukić, Robert Scott Young, Zifa Zuhair, James Parker, Inez Kesuma, Gargi Giri, Liam Bird, Alexander J. E. Rettie, Rhodri Jervis, James B. Robinson, Denis Cumming, Thomas S. Miller and Paul R. Shearing

Crack formation during electrode drying is a potential hindrance to the manufacture of high energy density electrodes. In this study, highly sensitive digital volume correlation is used to identify the precise moment of crack initiation.

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